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Tropospheric distribution of ozone and its precursors over the tropical Indian Ocean

Identifieur interne : 000188 ( PascalFrancis/Corpus ); précédent : 000187; suivant : 000189

Tropospheric distribution of ozone and its precursors over the tropical Indian Ocean

Auteurs : N. Saraf ; G. Beig ; M. Schultz

Source :

RBID : Pascal:04-0267728

Descripteurs français

English descriptors

Abstract

To evaluate the atmospheric ozone measurements of the Indian Ocean during the dry winter season from January to March, an analysis of ozone and its precursors has been made using the Model of Ozone and its Related Tracers (MOZART-2), a global chemical transport model. The ozonesonde measurements were made on board the ship Sagar Kanya during the Indian Ocean Experiment 1999 (INDOEX-99), which covered the region from 11.3°N to 20.2°S and from 62.3°E to 75.8°E. These measurements reveal surface ozone values on the order of 20-50 ppb over the oceanic region and increasing concentrations in the midtroposphere in the range 50-100 ppb, followed by a steep gradient (>120 ppb) near the tropopause. The model qualitatively reproduces most of the broad features observed in the ozonesonde measurements. The low value of O3 over the ocean is characterized by the low concentration of NOx and CO as simulated by the model, but the relationship between O3 and NOx breaks down toward the continent where NOx increases sharply and O3 does not follow the steep gradient. The variation in CO from ocean to continent is closely related to the O3 variation. The model reproduces the latitudinal variation of CO in this region well but underestimates the CO concentration by 30-50%, probably because of underestimated emission values. The latitudinal distribution of ozone over the marine boundary layer shows a decrease from north of the equator to the south as the CO-rich air from the continent spreads toward the ocean, thereby reflecting the inflow of pollutants to the pristine marine region during the dry winter season.

Notice en format standard (ISO 2709)

Pour connaître la documentation sur le format Inist Standard.

pA  
A01 01  1    @0 0148-0227
A03   1    @0 J. geophys. res.
A05       @2 108
A06       @2 D20
A08 01  1  ENG  @1 Tropospheric distribution of ozone and its precursors over the tropical Indian Ocean
A11 01  1    @1 SARAF (N.)
A11 02  1    @1 BEIG (G.)
A11 03  1    @1 SCHULTZ (M.)
A14 01      @1 Indian Institute of Tropical Meteorology @2 Pune @3 IND @Z 1 aut. @Z 2 aut.
A14 02      @1 Max-Planck-Institut für Meteorologie @2 Hamburg @3 DEU @Z 3 aut.
A20       @2 ACH4.1-ACH4.9
A21       @1 2003
A23 01      @0 ENG
A43 01      @1 INIST @2 3144 @5 354000118947490270
A44       @0 0000 @1 © 2004 INIST-CNRS. All rights reserved.
A45       @0 36 ref.
A47 01  1    @0 04-0267728
A60       @1 P
A61       @0 A
A64 01  1    @0 Journal of geophysical research
A66 01      @0 USA
C01 01    ENG  @0 To evaluate the atmospheric ozone measurements of the Indian Ocean during the dry winter season from January to March, an analysis of ozone and its precursors has been made using the Model of Ozone and its Related Tracers (MOZART-2), a global chemical transport model. The ozonesonde measurements were made on board the ship Sagar Kanya during the Indian Ocean Experiment 1999 (INDOEX-99), which covered the region from 11.3°N to 20.2°S and from 62.3°E to 75.8°E. These measurements reveal surface ozone values on the order of 20-50 ppb over the oceanic region and increasing concentrations in the midtroposphere in the range 50-100 ppb, followed by a steep gradient (>120 ppb) near the tropopause. The model qualitatively reproduces most of the broad features observed in the ozonesonde measurements. The low value of O3 over the ocean is characterized by the low concentration of NOx and CO as simulated by the model, but the relationship between O3 and NOx breaks down toward the continent where NOx increases sharply and O3 does not follow the steep gradient. The variation in CO from ocean to continent is closely related to the O3 variation. The model reproduces the latitudinal variation of CO in this region well but underestimates the CO concentration by 30-50%, probably because of underestimated emission values. The latitudinal distribution of ozone over the marine boundary layer shows a decrease from north of the equator to the south as the CO-rich air from the continent spreads toward the ocean, thereby reflecting the inflow of pollutants to the pristine marine region during the dry winter season.
C02 01  2    @0 220
C02 02  3    @0 001E
C03 01  2  FRE  @0 Troposphère @5 26
C03 01  2  ENG  @0 troposphere @5 26
C03 02  2  FRE  @0 Ozone @5 27
C03 02  2  ENG  @0 ozone @5 27
C03 02  2  SPA  @0 Ozono @5 27
C03 03  X  FRE  @0 Précurseur @5 28
C03 03  X  ENG  @0 Precursor @5 28
C03 03  X  SPA  @0 Precursor @5 28
C03 04  X  FRE  @0 Saison sèche @5 29
C03 04  X  ENG  @0 Dry season @5 29
C03 04  X  SPA  @0 Estación seca @5 29
C03 05  X  FRE  @0 Hiver @5 30
C03 05  X  ENG  @0 Winter @5 30
C03 05  X  SPA  @0 Invierno @5 30
C03 06  X  FRE  @0 Modèle chimique @5 31
C03 06  X  ENG  @0 Chemical model @5 31
C03 06  X  SPA  @0 Modelo químico @5 31
C03 07  2  FRE  @0 Traceur @5 32
C03 07  2  ENG  @0 tracers @5 32
C03 07  2  SPA  @0 Trazador @5 32
C03 08  X  FRE  @0 Tropopause @5 33
C03 08  X  ENG  @0 Tropopause @5 33
C03 08  X  SPA  @0 Tropopausa @5 33
C03 09  X  FRE  @0 Variation latitudinale @5 34
C03 09  X  ENG  @0 Latitudinal variation @5 34
C03 09  X  SPA  @0 Variación latitudinal @5 34
C03 10  X  FRE  @0 Répartition latitudinale @5 35
C03 10  X  ENG  @0 Latitudinal distribution @5 35
C03 10  X  SPA  @0 Distribución latitudinal @5 35
C03 11  X  FRE  @0 Atmosphère marine @5 36
C03 11  X  ENG  @0 Marine atmosphere @5 36
C03 11  X  SPA  @0 Atmósfera marina @5 36
C03 12  X  FRE  @0 Couche limite atmosphérique @5 37
C03 12  X  ENG  @0 Atmospheric boundary layer @5 37
C03 12  X  SPA  @0 Capa límite atmosférico @5 37
C03 13  2  FRE  @0 Océan Indien @5 46
C03 13  2  ENG  @0 Indian Ocean @5 46
C03 13  2  SPA  @0 Océano Indico @5 46
N21       @1 166
N44 01      @1 OTO
N82       @1 OTO

Format Inist (serveur)

NO : PASCAL 04-0267728 INIST
ET : Tropospheric distribution of ozone and its precursors over the tropical Indian Ocean
AU : SARAF (N.); BEIG (G.); SCHULTZ (M.)
AF : Indian Institute of Tropical Meteorology/Pune/Inde (1 aut., 2 aut.); Max-Planck-Institut für Meteorologie/Hamburg/Allemagne (3 aut.)
DT : Publication en série; Niveau analytique
SO : Journal of geophysical research; ISSN 0148-0227; Etats-Unis; Da. 2003; Vol. 108; No. D20; ACH4.1-ACH4.9; Bibl. 36 ref.
LA : Anglais
EA : To evaluate the atmospheric ozone measurements of the Indian Ocean during the dry winter season from January to March, an analysis of ozone and its precursors has been made using the Model of Ozone and its Related Tracers (MOZART-2), a global chemical transport model. The ozonesonde measurements were made on board the ship Sagar Kanya during the Indian Ocean Experiment 1999 (INDOEX-99), which covered the region from 11.3°N to 20.2°S and from 62.3°E to 75.8°E. These measurements reveal surface ozone values on the order of 20-50 ppb over the oceanic region and increasing concentrations in the midtroposphere in the range 50-100 ppb, followed by a steep gradient (>120 ppb) near the tropopause. The model qualitatively reproduces most of the broad features observed in the ozonesonde measurements. The low value of O3 over the ocean is characterized by the low concentration of NOx and CO as simulated by the model, but the relationship between O3 and NOx breaks down toward the continent where NOx increases sharply and O3 does not follow the steep gradient. The variation in CO from ocean to continent is closely related to the O3 variation. The model reproduces the latitudinal variation of CO in this region well but underestimates the CO concentration by 30-50%, probably because of underestimated emission values. The latitudinal distribution of ozone over the marine boundary layer shows a decrease from north of the equator to the south as the CO-rich air from the continent spreads toward the ocean, thereby reflecting the inflow of pollutants to the pristine marine region during the dry winter season.
CC : 220; 001E
FD : Troposphère; Ozone; Précurseur; Saison sèche; Hiver; Modèle chimique; Traceur; Tropopause; Variation latitudinale; Répartition latitudinale; Atmosphère marine; Couche limite atmosphérique; Océan Indien
ED : troposphere; ozone; Precursor; Dry season; Winter; Chemical model; tracers; Tropopause; Latitudinal variation; Latitudinal distribution; Marine atmosphere; Atmospheric boundary layer; Indian Ocean
SD : Ozono; Precursor; Estación seca; Invierno; Modelo químico; Trazador; Tropopausa; Variación latitudinal; Distribución latitudinal; Atmósfera marina; Capa límite atmosférico; Océano Indico
LO : INIST-3144.354000118947490270
ID : 04-0267728

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Pascal:04-0267728

Le document en format XML

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<div type="abstract" xml:lang="en">To evaluate the atmospheric ozone measurements of the Indian Ocean during the dry winter season from January to March, an analysis of ozone and its precursors has been made using the Model of Ozone and its Related Tracers (MOZART-2), a global chemical transport model. The ozonesonde measurements were made on board the ship Sagar Kanya during the Indian Ocean Experiment 1999 (INDOEX-99), which covered the region from 11.3°N to 20.2°S and from 62.3°E to 75.8°E. These measurements reveal surface ozone values on the order of 20-50 ppb over the oceanic region and increasing concentrations in the midtroposphere in the range 50-100 ppb, followed by a steep gradient (>120 ppb) near the tropopause. The model qualitatively reproduces most of the broad features observed in the ozonesonde measurements. The low value of O
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<s0>To evaluate the atmospheric ozone measurements of the Indian Ocean during the dry winter season from January to March, an analysis of ozone and its precursors has been made using the Model of Ozone and its Related Tracers (MOZART-2), a global chemical transport model. The ozonesonde measurements were made on board the ship Sagar Kanya during the Indian Ocean Experiment 1999 (INDOEX-99), which covered the region from 11.3°N to 20.2°S and from 62.3°E to 75.8°E. These measurements reveal surface ozone values on the order of 20-50 ppb over the oceanic region and increasing concentrations in the midtroposphere in the range 50-100 ppb, followed by a steep gradient (>120 ppb) near the tropopause. The model qualitatively reproduces most of the broad features observed in the ozonesonde measurements. The low value of O
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<s5>36</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA">
<s0>Atmósfera marina</s0>
<s5>36</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE">
<s0>Couche limite atmosphérique</s0>
<s5>37</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG">
<s0>Atmospheric boundary layer</s0>
<s5>37</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA">
<s0>Capa límite atmosférico</s0>
<s5>37</s5>
</fC03>
<fC03 i1="13" i2="2" l="FRE">
<s0>Océan Indien</s0>
<s5>46</s5>
</fC03>
<fC03 i1="13" i2="2" l="ENG">
<s0>Indian Ocean</s0>
<s5>46</s5>
</fC03>
<fC03 i1="13" i2="2" l="SPA">
<s0>Océano Indico</s0>
<s5>46</s5>
</fC03>
<fN21>
<s1>166</s1>
</fN21>
<fN44 i1="01">
<s1>OTO</s1>
</fN44>
<fN82>
<s1>OTO</s1>
</fN82>
</pA>
</standard>
<server>
<NO>PASCAL 04-0267728 INIST</NO>
<ET>Tropospheric distribution of ozone and its precursors over the tropical Indian Ocean</ET>
<AU>SARAF (N.); BEIG (G.); SCHULTZ (M.)</AU>
<AF>Indian Institute of Tropical Meteorology/Pune/Inde (1 aut., 2 aut.); Max-Planck-Institut für Meteorologie/Hamburg/Allemagne (3 aut.)</AF>
<DT>Publication en série; Niveau analytique</DT>
<SO>Journal of geophysical research; ISSN 0148-0227; Etats-Unis; Da. 2003; Vol. 108; No. D20; ACH4.1-ACH4.9; Bibl. 36 ref.</SO>
<LA>Anglais</LA>
<EA>To evaluate the atmospheric ozone measurements of the Indian Ocean during the dry winter season from January to March, an analysis of ozone and its precursors has been made using the Model of Ozone and its Related Tracers (MOZART-2), a global chemical transport model. The ozonesonde measurements were made on board the ship Sagar Kanya during the Indian Ocean Experiment 1999 (INDOEX-99), which covered the region from 11.3°N to 20.2°S and from 62.3°E to 75.8°E. These measurements reveal surface ozone values on the order of 20-50 ppb over the oceanic region and increasing concentrations in the midtroposphere in the range 50-100 ppb, followed by a steep gradient (>120 ppb) near the tropopause. The model qualitatively reproduces most of the broad features observed in the ozonesonde measurements. The low value of O
<sub>3</sub>
over the ocean is characterized by the low concentration of NO
<sub>x</sub>
and CO as simulated by the model, but the relationship between O
<sub>3</sub>
and NO
<sub>x</sub>
breaks down toward the continent where NO
<sub>x</sub>
increases sharply and O
<sub>3</sub>
does not follow the steep gradient. The variation in CO from ocean to continent is closely related to the O
<sub>3</sub>
variation. The model reproduces the latitudinal variation of CO in this region well but underestimates the CO concentration by 30-50%, probably because of underestimated emission values. The latitudinal distribution of ozone over the marine boundary layer shows a decrease from north of the equator to the south as the CO-rich air from the continent spreads toward the ocean, thereby reflecting the inflow of pollutants to the pristine marine region during the dry winter season.</EA>
<CC>220; 001E</CC>
<FD>Troposphère; Ozone; Précurseur; Saison sèche; Hiver; Modèle chimique; Traceur; Tropopause; Variation latitudinale; Répartition latitudinale; Atmosphère marine; Couche limite atmosphérique; Océan Indien</FD>
<ED>troposphere; ozone; Precursor; Dry season; Winter; Chemical model; tracers; Tropopause; Latitudinal variation; Latitudinal distribution; Marine atmosphere; Atmospheric boundary layer; Indian Ocean</ED>
<SD>Ozono; Precursor; Estación seca; Invierno; Modelo químico; Trazador; Tropopausa; Variación latitudinal; Distribución latitudinal; Atmósfera marina; Capa límite atmosférico; Océano Indico</SD>
<LO>INIST-3144.354000118947490270</LO>
<ID>04-0267728</ID>
</server>
</inist>
</record>

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